Neutron imaging has been demonstrated to be a powerful tool to measure the in situ water content of commercial proton exchange membrane fuel cells (PEMFCs) in two and three dimensions. The National Institute of Standards and Technology neutron imaging facility was designed to produce a high intensity, highly collimated neutron imaging beam to measure the water content of operating fuel cells. The details of the neutron optics and neutron detection are discussed in terms of the random uncertainty in measuring the liquid water thickness that is typical of operating PEMFCs.
Issue Section:
Research Papers
1.
Zawodzinsk
, T. A.
, Neeman
, M.
, Sillerud
, L. O.
, and Gottesfeld
, S.
, 1991, “Determination of Water Diffusion Coefficients in Perfluorosulfonate Ionomeric Membranes
,” J. Phys. Chem.
0022-3654, 95
, pp. 6040
–6044
.2.
Pasaogullari
, U.
, and Wang
, C. Y.
, 2004, “Liquid Water Transport in Gas Diffusion Layer of Polymer Electrolyte Fuel Cells
,” J. Electrochem. Soc.
0013-4651, 151
, pp. A399
–A406
.3.
Owejan
, J. P.
, Trabold
, T. A.
, Gagliardo
, J. J.
, Jacobson
, D. L.
, Carter
, R. N.
, Hussey
, D. S.
, and Arif
, M.
, 2007, “Voltage Instability in a Simulated Fuel Cell Stack Correlated to Cathode Water Accumulation
,” J. Power Sources
0378-7753, 171
, pp. 626
–633
.4.
He
, S.
, Kim
, S. H.
, and Mench
, M. M.
, 2006, “1D Transient Model for Frost Heave in Polymer Electrolyte Fuel Cells
,” J. Electrochem. Soc.
0013-4651, 154
, pp. B1024
–B1033
(2006).5.
Maeda
, M.
, Hamada
, H.
, Tejima
, G.
, Shiozawa
, M.
, and Isogai
, Y.
, 2007, “Analysis of Water Distribution in a Gas Diffusion Layer Using X-Ray Computed Tomography
,” Conference Proceedings, Electrochemical Society Meeting
, Washington, DC
, October.6.
Garzon
, F. H.
, Lau
, S. H.
, Davey
, J. R.
, and Borup
, R.
, 2007, “Micro and Nano X-Ray Tomography of PEM Fuel Cell Membranes After Transient Operation
,” ECS Trans.
1938-5862, 11
, p. 1139
.7.
Sinha
, P. K.
, Halleck
, P.
, and Wang
, C. Y.
, 2006, “Quantification of Liquid Water Saturation in a PEM Fuel Cell Diffusion Medium Using X-Ray Microtomography
,” Electrochem. Solid-State Lett.
1099-0062, 9
, pp. A344
–A348
.8.
Theodorakakos
, A.
, Ous
, T.
, Gavaises
, A.
, Nouri
, J. M.
, Nikolopoulos
, N.
, and Yanagilhara
, H.
, 2006, “Dynamics of Water Droplets Detached From Porous Surfaces of Relevance to PEM Fuel Cells
,” J. Colloid Interface Sci.
0021-9797, 300
, pp. 673
–687
.9.
Hickner
, M. A.
, Siegel
, N. P.
, Chen
, K. S.
, McBrayer
, D. N.
, Hussey
, D. S.
, Jacobson
, D. L.
, and Arif
, M.
, 2006, “Real-Time Imaging of Liquid Water in An Operating Proton Exchange Membrane Fuel Cell
,” J. Electrochem. Soc.
0013-4651, 153
, pp. A902
–A908
.10.
Grundl
, J. A.
, Gilliam
, D. M.
, Dudey
, N. D.
, and Popek
, R. J.
, 1975, “Measurement of Absolute Fission Rates
,” Nucl. Technol.
0029-5450, 25
, pp. 237
–257
.11.
Hecht
, E.
, 1998, Optics
, Addison Wesley Longman, Inc.
, Reading, MA
.12.
Barrett
, H. H.
, and Swindell
, W.
, 1981, Radiological Imagining
, Academic Press
, San Diego, CA
.13.
Geiger
, H.
, 1909, “On a Diffuse Reflection of the Alpha-Particles
,” Proc. R. Soc. London, Ser. A
1364-5021, 82
, pp. 495
–500
.14.
Spowart
, A. R.
, 1969, “Measurement of Absolute Scintillation Efficiency of Granular and Glass Neutron Scintillators
,” Nucl. Instrum. Methods
0029-554X, 75
, pp. 35
–42
.15.
Lehmann
, E. H.
, Frei
, G.
, Kuhne
, G.
, and Boillat
, P.
, 2007, “The Micro-Setup for Neutron Imaging: A Major Step Forward to Improve the Spatial Resolution
,” Nucl. Instrum. Methods Phys. Res. A
0168-9002, 576
, pp. 389
–396
.16.
Siegmund
, O. H. W.
, Vallerga
, J. V.
, Martin
, A.
, Feller
, B.
, Arif
, M.
, Hussey
, D. S.
, and Jacobson
, D. L.
2007, “A High Spatial Resolution Event Counting Neutron Detector Using Microchannel Plates and Cross Delay Line Readout
,” Nucl. Instrum. Methods Phys. Res. A
0168-9002, 579
, pp. 188
–191
.17.
Siegmund
, O. H. W.
, 2006, World Conference on Neutron Radiography
, Gaithersburg, MD
.19.
Edura
, Y.
, and Morishima
, N.
, 2004, “Cold and Thermal Neutron Scattering in Liquid Water: Cross-Section Model and Dynamics of Water Molecules
,” Nucl. Instrum. Methods Phys. Res. A
0168-9002, 534
, pp. 531
–543
.20.
Hussey
, D. S.
, Jacobson
, D. L.
, Arif
, M.
, Owejan
, J. P.
, Gagliardo
, J. J.
, and Trabold
, T. A.
, 2007, “Neutron Images of the Through-Plane Water Distribution of an Operating PEM Fuel Cell
,” J. Power Sources
0378-7753, 172
, pp. 225
–228
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by American Society of Mechanical Engineers
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